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Han, J.*; 内村 友宏*; 荒木 康史; Yoon, J.-Y.*; 竹内 祐太郎*; 山根 結太*; 金井 駿*; 家田 淳一; 大野 英男*; 深見 俊輔*
Nature Physics, 21 Pages, 2024/04
被引用回数：0量子状態の幾何学的構造を特徴づける基礎的な量として、「量子計量」と「ベリー曲率」が存在する。ベリー曲率は、凝縮系において多種の重要な現象に寄与することが知られている。一方、量子計量も新たなトポロジカル物理現象の起源となることが予想されているが、特に常温常圧下においては、その効果はほとんど探索されていない。本研究では、トポロジカルカイラル反強磁性体Mn
Snと白金の接合系を用い、界面でのナノスピン構造を介して、電子系の量子計量構造の制御に成功した。ベリー曲率ではなく量子計量特有の効果として、時間反転反対称でかつ電子散乱に対して頑強な、二次非線形ホール効果を測定した。更に、界面スピン構造は弱磁場及び界面スピン軌道相互作用によって急峻に変調されるため、量子計量構造も鋭敏に制御可能であることを示した。本研究成果により、量子状態に内在する量子計量構造を活用したトポロジカル物理現象が室温環境下でも可能になり、且つ応用面においても非線形素子を構築する助けとなることが期待される。
Lee, S.*; 仲田 光樹; Tchernyshyov, O.*; Kim, S. K.*
Physical Review B, 107(18), p.184432_1 - 184432_12, 2023/05
被引用回数：5 パーセンタイル：87.72(Materials Science, Multidisciplinary)超対称量子力学に基づき、反強磁性スカーミオン構造を有する磁壁中のマグノンのトポロジカル量子輸送物性を明らかにする。スカーミオン型の磁気構造を有する磁壁中を伝搬するマグノンは、一種のゲージ場として作用する有効磁場を獲得する。そこで、この有効磁場中でのマグノンの反射・屈折現象を超対称量子力学に基づいて解析し、その伝搬および束縛マグノン状態を明らかにする。そして、ラウダウアー公式を用いて、磁壁のカイラリティが増加するにつれてマグノンによる熱流が減少することを明らかにする。本研究はスピンホール効果を活用した熱流の制御方法を理論的に提案する。
佐藤 哲也*; 加藤 岳生*; 大上 能悟*; 松尾 衛
Physical Review B, 107(18), p.L180406_1 - L180406_6, 2023/05
被引用回数：1 パーセンタイル：49.29(Materials Science, Multidisciplinary)We examine the mechanical rotation of a levitated magnetic particle that is induced by ferromagnetic resonance under microwave irradiation. We show that two stable solutions appear in a certain range of parameters by bifurcation when the rotation frequency is comparable to the microwave frequency. This phenomenon originates from the coexistence of the Barnett and the Einstein-de Haas effects. We also reveal that this measurement is sensitive to the strength of the spin-rotation coupling. Our work provides a platform for accessing a microscopic relaxation process from spin to macroscopic rotation.
佐野 涼太郎*; 松尾 衛
Physical Review Letters, 130(16), p.166201_1 - 166201_7, 2023/04
被引用回数：1 パーセンタイル：0(Physics, Multidisciplinary)Recent experiments have shown an indication of a hydrodynamic magnon behavior in ultrapure ferromagnetic insulators; however, its direct observation is still lacking. Here, we derive a set of coupled hydrodynamic equations and study the thermal and spin conductivities for such a magnon fluid. We reveal the drastic breakdown of the magnonic Wiedemann-Franz law as a hallmark of the hydrodynamics regime, which will become key evidence for the experimental realization of an emergent hydrodynamic magnon behavior. Therefore, our results pave the way toward the direct observation of magnon fluids.
Sn nanodot佐藤 佑磨*; 竹内 祐太郎*; 山根 結太*; Yoon, J.-Y.*; 金井 駿*; 家田 淳一; 大野 英男*; 深見 俊輔*
Applied Physics Letters, 122(12), p.122404_1 - 122404_5, 2023/03
被引用回数：2 パーセンタイル：49.29(Physics, Applied)
-MnSn, an antiferromagnet having a non-collinear spin structure in a kagome lattice, has attracted great attention owing to various intriguing properties such as large anomalous Hall effect. Stability of magnetic state against thermal fluctuation, characterized in general by the thermal stability factor 
, has been well studied in ferromagnetic systems but not for antiferromagnets. Here we study of the antiferromagnetic MnSn nanodots as a function of their diameter 
. To obtain , we measure the switching probability as a function of pulse-field amplitude and analyze the results based on a model developed by accounting for two and six-fold magnetic anisotropies in the kagome plane. We observe no significant change in down to 
nm below which it decreases with . The obtained dependence is well explained by a single-domain and nucleation-mediated reversal models. These findings provide a basis to understand the thermal fluctuation and reversal mechanism of antiferromagnets for device application.
仲田 光樹; 鈴木 渓
Physical Review Letters, 130(9), p.096702_1 - 096702_6, 2023/03
被引用回数：3 パーセンタイル：76.59(Physics, Multidisciplinary)量子場の真空ゆらぎによって創発されるカシミア効果は、古典力学には対応物が存在しないという意味において真に量子力学的な効果である。しかし、カシミア効果はこれまでフォトン(光子)を舞台に研究されており、磁性体中でのカシミア効果、特にそのカシミアエネルギーの膜厚依存性については十分な理解は得られていない。そこで本研究では格子場の理論の観点から、磁性絶縁体中のスピン波を量子化したマグノンに着目し、マグノン量子場により創発されるカシミア効果「マグノン・カシミア効果」及びその膜厚依存性を明らかにする。更に反強磁性絶縁体だけでなくフェリ磁性絶縁体(例:YIG)においてもマグノン・カシミア効果が創発することを示し、スピントロニクス分野で中心的な役割を担うYIGがカシミア効果の工学的応用を目指すカシミアエンジニアリング分野にとっても絶好の舞台であることを明らかにする。本研究は、マグノン・カシミアエンジニアリングの基礎学理の構築に大きく貢献することが期待される。
BaCo(PO
)Sheng, J.*; Wang, L.*; Candini, A.*; Jiang, W.*; Huang, L.*; Xi, B.*; Zhao, J.*; Ge, H.*; Zhao, N.*; Fu, Y.*; et al.
Proceedings of the National Academy of Sciences of the United States of America, 119(51), p.e2211193119_1 - e2211193119_9, 2022/12
被引用回数：4 パーセンタイル：56.47(Multidisciplinary Sciences)Although considerable progress has been made in the theoretical understanding of the low-dimensional frustrated quantum magnets, experimental realizations of a well-established scaling analysis are still scarce. This is particularly true for the two-dimensional antiferromagnetic triangular lattices. Owing to the small exchange strength, the newly discovered compound NaBaCo(PO) provides a rare opportunity for clarifying the quantum criticality in an ideal triangular lattice with quantum spin S=1/2. In addition to the establishment of the complete phase diagrams, the spin Hamiltonian with a negligible interplane interaction has been determined through the spin wave dispersion in the polarized state, which is consistent with the observation of a two-dimensional quantum critical point with the Bose-Einstein condensation of diluted free bosons.
Sn thin films by magneto-optical Kerr effect内村 友宏*; Yoon, J.-Y.*; 佐藤 佑磨*; 竹内 祐太郎*; 金井 駿*; 武智 涼太*; 岸 桂輔*; 山根 結太*; DuttaGupta, S.*; 家田 淳一; et al.
Applied Physics Letters, 120(17), p.172405_1 - 172405_5, 2022/04
被引用回数：11 パーセンタイル：84.45(Physics, Applied)We perform a hysteresis-loop measurement and domain imaging for 
-oriented -Mn
Sn
thin films using magneto-optical Kerr effect (MOKE) and compare it with the anomalous Hall effect (AHE) measurement. We obtain a large Kerr rotation angle of 10 mdeg., comparable with bulk single-crystal MnSn. The composition 
dependence of AHE and MOKE shows a similar trend, suggesting the same origin, i.e., the non-vanishing Berry curvature in the momentum space. Magnetic domain observation at the saturated state shows that x dependence of AHE and MOKE is explained by an amount of reversible area that crucially depends on the crystalline structure of the film. Furthermore, in-depth observation of the reversal process reveals that the reversal starts with nucleation of sub-micrometer-scale domains dispersed in the film, followed by a domain expansion, where the domain wall preferentially propagates along the ![$$[11bar{2}0]$$](/search/images/ERNTCMK2MJQXE4ZSPUYF0JA.gif)
direction. Our study provides a basic understanding of the spatial evolution of the reversal of chiral-spin structure in non-collinear antiferromagnetic thin films.
-edge EXAFS and magnetic EXAFS studies on the halfmetallic ferromagnet CoMnSi向後 純也*; 藤原 秀紀*; 関山 明*; 斎藤 祐児; 梅津 理恵*; 二木 かおり*
Journal of the Physical Society of Japan, 91(3), p.034702_1 - 034702_12, 2022/03
被引用回数：0 パーセンタイル：0(Physics, Multidisciplinary)We report magnetic circular dichroism in extended X-ray absorption fine structure (EXAFS) in a prototypical halfmetallic ferromagnet, CoMnSi. The EXAFS oscillations at the Mn L edges are analyzed to obtain parameters used in the analysis of the magnetic EXAFS (MEXAFS). Theoretical calculations of MEXAFS spectra in CoMnSi show that the linear-path scatterings have larger contributions than the multiple triangular-path scatterings. Furthermore, the period of the oscillations in the MEXAFS spectra is shorter than that in the EXAFS spectra indicating that the far site contributions from the second to the fourth nearest neighbor Co and the third nearest Si atoms can strongly influence the MEXAFS oscillations, while the Mn atoms, despite the large magnetic moment, can have little contributions due to the interference of the spin components.
Schreiber, F.*; Meer, H.*; Schmitt, C.*; Ramos, R.*; 齊藤 英治; Baldrati, L.*; Kl
ui, M.*
Physical Review Applied (Internet), 16(6), p.064023_1 - 064023_9, 2021/12
被引用回数：3 パーセンタイル：26.56(Physics, Applied)We analyze the complex impact of the local magnetic spin texture on the transverse Hall-type voltage in device structures utilized to measure magnetoresistance effects. We find a highly localized and asymmetric magnetic sensitivity in the eight-terminal geometries that are frequently used in current-induced switching experiments, for instance, to probe antiferromagnetic materials. Using current-induced switching of antiferromagnetic NiO/Pt as an example, we estimate the change in the spin Hall magnetoresistance signal associated with switching events based on the domain-switching patterns observed via direct imaging. This estimate correlates with the actual electrical data after subtraction of a nonmagnetic contribution. Here, the consistency of the correlation across three measurement geometries with fundamentally different switching patterns strongly indicates a magnetic origin of the measured and analyzed electrical signals.
竹内 祐太郎*; 山根 結太*; Yoon, J.-Y.*; 伊藤 隆一*; 陣内 佛霖*; 金井 駿*; 家田 淳一; 深見 俊輔*; 大野 英男*
Nature Materials, 20(10), p.1364 - 1370, 2021/10
被引用回数：84 パーセンタイル：98.68(Chemistry, Physical)Electrical manipulation of magnetic materials by current-induced spin torque constitutes the basis of spintronics. Recent studies have demonstrated electrical controls of ferromagnets and collinear antiferromagnets by spin-orbit torque (SOT). Here we show an unconventional response to SOT of a non-collinear antiferromagnet, which has recently attracted great attention owing to large anomalous Hall effect despite vanishingly small net magnetization. In heterostructures with epitaxial non-collinear antiferromagnet MnSn, we observe a characteristic fluctuation of Hall resistance, which is attributed to a persistent rotation of chiral-spin structure of MnSn driven by SOT. We find that level of the fluctuation that varies with sample size represents the number of magnetic domains of MnSn. In addition, MnSn thickness dependence of critical current reveals that SOT generated by small current density below 20 MA cm
effectively acts on the chiral-spin structure even in thick MnSn above 20 nm. The results provide unprecedented pathways of electrical manipulation of magnetic materials, offering new-concept spintronics devices with unconventional functionalities and low-power consumption.
Mg
TiO社本 真一; 山内 宏樹; 池内 和彦*; Lee, M. K.*; Chang, L.-J.*; Garlea, V. O.*; Hwang, I. Y.*; Lee, K. H.*; Chung, J.-H.*
Journal of the Physical Society of Japan, 90(9), p.093703_1 - 093703_4, 2021/09
被引用回数：0 パーセンタイル：0(Physics, Multidisciplinary)ハニカム格子反強磁性体MnMgTiOの5T磁場下でのスピンフロップ相の磁気構造を弾性散乱と非弾性散乱を相補的に用いることで、初めて提案した。
Sn thin filmsYoon, J.-Y.*; 竹内 祐太郎*; DuttaGupta, S.*; 山根 結太*; 金井 駿*; 家田 淳一; 大野 英男*; 深見 俊輔*
AIP Advances (Internet), 11(6), p.065318_1 - 065318_6, 2021/06
被引用回数：14 パーセンタイル：78.56(Nanoscience & Nanotechnology)We investigate the relationship between structural parameters, magnetic ordering, and the anomalous Hall effect (AHE) of MnSn (
) thin films annealed at various temperature 
. The crystal structure changes with and and at 
C near the stoichiometric composition (
) epitaxial single-phase 0
-MnSn(
) is obtained. At room temperature, a larger AHE is obtained when the single-phase epitaxial MnSn with the lattice constant closer to that of bulk is formed. The temperature dependence of the AHE shows different behaviors depending on and can be explained by considering the variation of magnetic ordering. A close inspection into the temperature and composition dependence suggests a variation of magnetic phase transition temperature with composition and/or a possible correlation between the AHE and Fermi level position with respect to the Weyl points. Our comprehensive study would provide the basis for utilizing the unique functionalities of non-collinear antiferromagnetic materials.
Hwang, I. Y.*; Lee, K. H.*; Chung, J.-H.*; 池内 和彦*; Garlea, V. O.*; 山内 宏樹; 赤津 光洋*; 社本 真一
Journal of the Physical Society of Japan, 90(6), p.064708_1 - 064708_6, 2021/06
被引用回数：2 パーセンタイル：29.32(Physics, Multidisciplinary)ハニカム格子反強磁性体MnTiOのスピン波を調べ、スピン間の交換相互作用を正確に求めた。
Jiang, N.*; 新居 陽一*; 有沢 洋希*; 齊藤 英治; 大江 純一郎*; 小野瀬 佳文*
Physical Review Letters, 126(17), p.177205_1 - 177205_5, 2021/04
被引用回数：4 パーセンタイル：48.26(Physics, Multidisciplinary)Chirality in a helimagnetic structure is determined by the sense of magnetic moment rotation. We found that the chiral information did not disappear even after the phase transition to the high-temperature ferromagnetic phase in a helimagnet MnP. The 2nd harmonic resistivity 
, which reflects the breaking down of mirror symmetry, was found to be almost unchanged after heating the sample above the ferromagnetic transition temperature and cooling it back to the helimagnetic state. The application of a magnetic field along the easy axis in the ferromagnetic state quenched the chirality-induced . This indicates that the chirality memory effect originated from the ferromagnetic domain walls.
Si; 
Si NMR study酒井 宏典; 松本 裕司*; 芳賀 芳範; 徳永 陽; 神戸 振作
Physical Review B, 103(8), p.085114_1 - 085114_8, 2021/02
被引用回数：0 パーセンタイル：0(Materials Science, Multidisciplinary)重い電子系反強磁性体CeRhSiにおいて、Si核核磁気共鳴(NMR)を用いて、圧力下相図について微視的に調べた。NMRデータから、反強磁性伝搬ベクトル
に依らない単一サイト近藤効果の特徴的温度スケール
を導出した。圧力下の反強磁性臨界点においての発散的異常は見られず、重い電子系の典型的なDoniach描像と矛盾しない結果が得られた。
Meer, H.*; Schreiber, F.*; Schmitt, C.*; Ramos, R.*; 齊藤 英治; Gomonay, O.*; Sinova, J.*; Baldrati, L.*; Klui, M.*
Nano Letters, 21(1), p.114 - 119, 2021/01
被引用回数：54 パーセンタイル：96.96(Chemistry, Multidisciplinary)We unravel the origin of current-induced magnetic switching of insulating antiferromagnet/heavy metal systems. We utilize concurrent transport and magneto-optical measurements to image the switching of antiferromagnetic domains in specially engineered devices of NiO/Pt bilayers. Different electrical pulsing and device geometries reveal different final states of the switching with respect to the current direction. We can explain these through simulations of the temperature-induced strain, and we identify the thermomagnetoelastic switching mechanism combined with thermal excitations as the origin, in which the final state is defined by the strain distributions and heat is required to switch the antiferromagnetic domains. We show that such a potentially very versatile noncontact mechanism can explain the previously reported contradicting observations of the switching final state, which were attributed to spin-orbit torque mechanisms.
森 道康
Journal of the Physical Society of Japan, 89(11), p.114705_1 - 114705_7, 2020/11
被引用回数：1 パーセンタイル：11.81(Physics, Multidisciplinary)The nuclear magnetic relaxation time 
in a ferrimagnetic insulators is calculated within the mean-field approximation for the magnetic exchange interactions and the Raman process involving the hyperfine interaction. We find that the value of 1/ on one type of site increases rapidly near the compensation temperature , whereas that on the other type of site does not increase up to Curie temperature 
. This is due to the fact that the soft-magnon bandwidth becomes comparable to . An increase in 1/ below is found also in another type ferrimagnet, which shows a hump structure in the temperature dependence of magnetization instead of compensation. Also in that case, we find the rapid increase in 1/ below , even though the magnetization does not show compensation. The coexistence of soft and hard magnons leads to these remarkable properties of ferrimagnets.
Baldrati, L.*; Schmitt, C.*; Gomonay, O.*; Lebrun, R.*; Ramos, R.*; 齊藤 英治; Sinova, J.*; Klui, M.*
Physical Review Letters, 125(7), p.077201_1 - 077201_6, 2020/08
被引用回数：36 パーセンタイル：91.52(Physics, Multidisciplinary)We achieve current-induced switching in collinear insulating antiferromagnetic CoO/Pt, with fourfold in-plane magnetic anisotropy. This is measured electrically by spin Hall magnetoresistance and confirmed by the magnetic field-induced spin-flop transition of the CoO layer. By applying current pulses and magnetic fields, we quantify the efficiency of the acting current-induced torques and estimate a current-field equivalence ratio of 
TA
m
. The N
el vector final state 
is in line with a thermomagnetoelastic switching mechanism for a negative magnetoelastic constant of the CoO.
藤原 理賀*; 森田 克洋*; Mole, R.*; 満田 節生*; 遠山 貴巳*; 矢野 真一郎*; Yu, D.*; 曽田 繁利*; 桑井 智彦*; 幸田 章宏*; et al.
Nature Communications (Internet), 11, p.3429_1 - 3429_7, 2020/07
被引用回数：39 パーセンタイル：92.14(Multidisciplinary Sciences)Observation of a quantum spin liquid (QSL) state is one of the most important goals in condensed-matter physics, as well as the development of new spintronic devices that support next-generation industries. The QSL in two-dimensional quantum spin systems is expected to be due to geometrical magnetic frustration, and thus a kagome-based lattice is the most probable playground for QSL. Here, we report the first experimental results of the QSL state on a square-kagome quantum antiferromagnet, KCu
AlBiO
(SO)
Cl. Comprehensive experimental studies via magnetic susceptibility, magnetisation, heat capacity, muon spin relaxation, and inelastic neutron scattering measurements reveal the formation of a gapless QSL at very low temperatures close to the ground state. The QSL behavior cannot be explained fully by a frustrated Heisenberg model with nearest-neighbor exchange interactions, providing a theoretical challenge to unveil the nature of the QSL state.
